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Probing the influence of dielectric environment on excitons in monolayer WSe2: Insight from high magnetic fields

机译:探讨介电环境对单层激子的影响   Wse2:高磁场的洞察力

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摘要

Excitons in atomically-thin semiconductors necessarily lie close to asurface, and therefore their properties are expected to be strongly influencedby the surrounding dielectric environment. However, systematic studiesexploring this role are challenging, in part because the most readilyaccessible exciton parameter -- the exciton's optical transition energy -- islargely \textit{un}affected by the surrounding medium. Here we show that therole of the dielectric environment is revealed through its systematic influenceon the \textit{size} of the exciton, which can be directly measured via thediamagnetic shift of the exciton transition in high magnetic fields. Usingexfoliated WSe$_2$ monolayers affixed to single-mode optical fibers, we tunethe surrounding dielectric environment by encapsulating the flakes withdifferent materials, and perform polarized low-temperature magneto-absorptionstudies to 65~T. The systematic increase of the exciton's size with dielectricscreening, and concurrent reduction in binding energy (also inferred from thesemeasurements), is quantitatively compared with leading theoretical models.These results demonstrate how exciton properties can be tuned in future 2Doptoelectronic devices.
机译:原子薄半导体中的激子必定靠近表面,因此,其性能预计会受到周围介电环境的强烈影响。但是,探索这种作用的系统研究具有挑战性,部分原因是最容易获得的激子参数-激子的光学跃迁能-在很大程度上不受周围介质的影响。在这里,我们表明介电环境的作用是通过其对激子的\ textit {size}的系统影响而揭示的,可以通过在高磁场中激子跃迁的反磁性位移直接测量。我们使用附着在单模光纤上的片状WSe $ _2 $单层,通过用不同的材料封装薄片来调谐周围的介电环境,并进行极化的低温磁吸收研究,达到65〜T。与领先的理论模型定量地比较了通过介电屏蔽系统激子尺寸的系统增加以及结合能的同时降低(也可以从这些测量中推断出),这些结果证明了如何在未来的2掺杂电子器件中调节激子性质。

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